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2004
Other 6-membered heterocycles
R 0670
Rh-Catalyzed Amination of Ethereal Cα—H Bonds: A Versatile Strategy for the
of Complex Amines. — Recently reported N,O-acetals, e.g. type (II), pre50- 135 Synthesis
pared by Rh-catalyzed amination of etheral Cα—H bonds, are utilized for the first time
in allyl addition reactions. They give stereoselective access to a wide range of synthetically interesting oxathiazinane derivatives. The stereochemical outcome of these reactions can be predicted based on Stevens/Felkin—Anh transition state analysis. —
(FIORI, K. W.; FLEMING, J. J.; DU BOIS*, J.; Angew. Chem., Int. Ed. 43 (2004) 33,
4349-4352; Dep. Chem., Stanford Univ., Stanford, CA 94305, USA; Eng.) —
Nuesgen
2004
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