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2005
Carboxylic acid esters
P 0360
Enantioselective Synthesis of Acyclic Allylic Esters Catalyzed by a Palladium/
System. — The synthesis of chiral nonracemic acyclic allylic pivalates via
02- 062 BINAP(S)
the Pd-catalyzed allylic substitution of racemic carbonates is presented. Good to high
enantioselectivities are observed in several cases. A significant kinetic resolution of the
1,3-dimethylallyl substrate (I) is also observed leading to the formation of esters of both
enantiomers of an allylic alcohol. — (FALLER*, J. W.; WILT, J. C.; Tetrahedron
Lett. 45 (2004) 41, 7613-7616; Dep. Chem., Yale Univ., New Haven, CT 06520, USA;
Eng.) — M. Paetzel
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