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2005
Rearrangements
O 0140
Asymmetric Allylic Alkylation of Ketone Enolates: An Asymmetric Claisen Sur— The high levels of asymmetric induction are shown to be obtained in the
06- 050 rogate.
palladium-catalyzed decarboxylative rearrangement of allyl-β-keto carboxylates. The
reaction is most effective in the presence of a mixture of catalytic palladium(0) and
Trost ligand and leads to the regiospecific generation of enolates under extremely mild
conditions. — (BURGER, E. C.; TUNGE*, J. A.; Org. Lett. 6 (2004) 22, 4113-4115;
Dep. Chem., Univ. Kans., Lawrence, KS 66045, USA; Eng.) — Steudel
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