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2005
Oxidation
O 0212
08- 045
Nitrous Oxide Oxidation Catalyzed by Ruthenium Porphyrin Complex. — Olefins, primary, secondary, and benzylic alcohols are smoothly oxidized to their corresponding epoxides, aldehydes and ketones in the presence of dioxoruthenium tetramesitylprophyrin complex using dinitrogen oxide as an oxidant. In the case of dihydroanthracenes (VII), anthraquinones and anthracenes are obtained by competitive
reactions. Regulation of the reaction conditions leads to selective production of either
anthraquinones (VIII) or anthracenes (IX). — (TANAKA, H.; HASHIMOTO, K.;
SUZUKI, K.; KITAICHI, Y.; SATO, M.; IKENO, T.; YAMADA*, T.; Bull. Chem.
Soc. Jpn. 77 (2004) 10, 1905-1914; Dep. Chem., Fac. Sci. Technol., Keio Univ.,
Kohoku, Yokohama 223, Japan; Eng.) — H. Hoennerscheid
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