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2005
Aziridine derivatives
R 0040
Design of a Robust Ru(salen) Complex: Aziridination with Improved Turnover
Using N-Arylsulfonyl Azides as Precursors. — A new robust fluorinated
11- 120 Number
(OC)Ru(salen) complex is designed on the basis of the X-ray structure of its parent
complex to show improved turnover numbers (up to 878) and enantioselectivities
(up to 99%) in aziridination reactions using tosyl- or nitrobenzensulfonyl (Nos) azide
as the nitrene precursor. The latter is synthetically advantageous since the Nos-group
can be removed under mild conditions. — (OMURA, K.; UCHIDA, T.; IRIE, R.;
KATSUKI*, T.; Chem. Commun. (Cambridge) 2004, 18, 2060-2061; Dep. Chem.,
Fac. Sci., Kyushu Univ., Higashi, Fukuoka 812, Japan; Eng.) — M. Paetzel
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