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2005
Organo-silicon compounds
S 0060
Unusual Palladium-Catalyzed Silaboration of Allenes Using Organic Iodides as
Mechanism and Application. — The reaction offers a new and general
23- 177 Initiators:
approach to 2-silylallylboronates and proceeds with excellent regio- and stereoselectivity via an unusual three-component assembling pathway. The products are totally
different in regiochemistry from those reported previously using Pd-catalysts without
organic iodides. Based on this reaction, a new stereoselective one-pot formation of
homoallylic alcohols of type (VII) is developed. — (CHANG, K.-J.; RAYABARAPU,
D. K.; YANG, F.-Y.; CHENG*, C.-H.; J. Am. Chem. Soc. 127 (2005) 1, 126-131;
Dep. Chem., Natl. Tsing Hua Univ., Hsinchu 30043, Taiwan; Eng.) — Jannicke
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