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2005
Indole derivatives
R 0140
Stereocontrolled Synthesis of Angularly Substituted 1-Azabicyclic Rings by Cat2-Aza-Cope Rearrangements. — The highly endothermic cationic 2-aza-Cope
30- 100 ionic
rearrangement of ketone-derived iminium ions is directed by subsequent methylene
transfer. Amine products containing a fully substituted carbon adjacent to nitrogen are
formed. In this way, a variety of bicyclic compounds with an angular allyl substitution
is prepared. — (ARON, Z. D.; OVERMAN*, L. E.; Org. Lett. 7 (2005) 5, 913-916;
Dep. Chem., Univ. Calif., Irvine, CA 92697, USA; Eng.) — R. Steudel
2005
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