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2005
Ketone derivatives
Q 0370
Cp*Ru(PN) Complex-Catalyzed Isomerization of Allylic Alcohols and Its Applito the Asymmetric Synthesis of Muscone (XI). — An efficient isomerization
37- 073 cation
of allylic alcohols into saturated carbonyl compounds is accomplished in the presence
of KOtBu using a new Ru-catalyst system under mild conditions. The method tolerates
a variety of functional groups and is even applicable to the asymmetric isomerization
of racemic sec-allylic alcohols with a prochiral olefin via dynamic kinetic resolution.
— (ITO, M.; KITAHARA, S.; IKARIYA*, T.; J. Am. Chem. Soc. 127 (2005) 17,
6172-6173; Dep. Appl. Chem., Tokyo Inst. Technol., Meguro, Tokyo 152, Japan;
Eng.) — S. Adam
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